Voldemort
Classy actor Ralph Fiennes brought the most evil wizard in the Harry Potter universe to life. The most extensive part of his transformation into He Who Must Not Be Named was the CGI removal of his nose in favor of snake-like slits. The rest of his makeup, like his claw-like hands and pallor skin, was real.
Thanos
The lead villain in the entire Marvel universe, Thanos, comes crashing down in Avengers: Endgame. With the capture of all the infinity stones, he could erase the entire universe with the snap of his fingers. He's played by Josh Brolin who, despite all that CGI, still somehow resembles the super villain.
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